Graphene oxide as efficient high-concentration formaldehyde scavenger and reutilization in supercapacitor | |
Department | 先进润滑与防护材料研究发展中心 |
Liang HY(梁红玉)1,2; Bu YF(卜永锋)1; Zhang YT(张雨田)3; Zhang JY(张俊彦)1; Zhang JY(张俊彦) | |
The second department | 固体润滑国家重点实验室 |
2015 | |
Source Publication | Journal of Colloid and Interface Science |
ISSN | 0021-9797 |
Volume | 444Pages:109-114 |
Abstract | Graphene oxide (GO) was investigated as a low-cost and high-efficient scavenger for high-concentration formaldehyde in alkali media. It showed very high removal capacity, 411 mg of formaldehyde per milligram of GO, and strong resistant to temperature changes. Additionally, the used GO can be easily renewed by a simple electrochemical method. By analyzing the componential and electrochemical characterizations of GO before and after use, the results showed that the degradation mechanism of formaldehyde is a collaborative process of chemical oxidation and physical adsorption, and the former dominates the degradation process. With the aid of oxygen-containing groups in GO, most formaldehyde can be easily oxidized by GO in alkaline media (this is equivalent to GO was reduced by formaldehyde). On the other hand, the used GO (reduced GO, noted as rGO) exhibits more ideal electronic double-layer capacitor (EDLC) feature than GO, along with higher rate capacitance (up to 136 F g_1 at 50 A g_1). In short, GO is not only an efficient formaldehyde scavenger, but the used GO (rGO) can serve as promising electrical energy storage material. This study provides new insights for us to reutilize the discarded adsorbents generated from the environmental protection. |
Keyword | Graphene Oxide High-concentration Formaldehyde Degradation Efficiency Chemical Oxidation Physical Adsorption Supercapacitor |
Subject Area | 材料科学与物理化学 |
DOI | 10.1016/j.jcis.2014.12.063 |
Funding Organization | National Natural Science Foundation of China (51205383;51305434) |
Indexed By | SCI |
If | 3.782 |
Language | 英语 |
Funding Project | 纳米润滑研究组 |
compositor | 第一作者单位 |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.licp.cn/handle/362003/7219 |
Collection | 中国科学院材料磨损与防护重点实验室/先进润滑与防护材料研究发展中心 固体润滑国家重点实验室(LSL) |
Corresponding Author | Zhang JY(张俊彦) |
Affiliation | 1.Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Lanzhou 1 Senior High Sch Gansu, Lanzhou 730030, Peoples R China |
Recommended Citation GB/T 7714 | Liang HY,Bu YF,Zhang YT,et al. Graphene oxide as efficient high-concentration formaldehyde scavenger and reutilization in supercapacitor[J]. Journal of Colloid and Interface Science,2015,444:109-114. |
APA | Liang HY,Bu YF,Zhang YT,Zhang JY,&张俊彦.(2015).Graphene oxide as efficient high-concentration formaldehyde scavenger and reutilization in supercapacitor.Journal of Colloid and Interface Science,444,109-114. |
MLA | Liang HY,et al."Graphene oxide as efficient high-concentration formaldehyde scavenger and reutilization in supercapacitor".Journal of Colloid and Interface Science 444(2015):109-114. |
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