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Efficient degradation of rhodamine B with magnetically separable Ag3PO4@MgFe2O4 composites under visible irradiation
Department环境材料与生态化学研究发展中心
Zhou TH(周添红)1,2; Zhang, Guozhen1; Ma PJ(马鹏军)2; Qiu XL(邱晓莉)2; Zhang, Hongwei1,3; Yang, Hao1; Liu G(刘刚)2
2018
Source PublicationJournal of Alloys and Compounds
ISSN0925-8388
Volume735Issue:0Pages:1277-1290
Abstract

 composites were successfully prepared via an ion-exchange deposition process. With Rhodmine B (RhB) as the model organic pollutant, Ag3PO4@MgFe2O4 system exhibited much superior degradation performance and stability, which was comparative to Ag3PO4 and MgFe2O4 system. The characterization results showed that Ag3PO4@MgFe2O4(10%) possessed high dispersion, large pore size (∼24 nm), larger transient photocurrent and longer fluorescence lifetime (∼10.83 ns). Furthermore, the effect of various parameters, such as temperature, initial pH, RhB concentration and catalyst loading on the RhB degradation were discussed in detail. Characterization results further indicate the MgFe2O4 over Ag3PO4 surface can inhibit Ag3PO4 from photocorrosion. Comparing the activity results dependence with the characterization results, it was indicated that the dependence of the photocatalytic activity on the efficient separation of photogenerated h+-e- pairs. This result indicates that the Ag3PO4@MgFe2O4(10%) catalyst can be a promising candidate for organic dyes degradation in waste water.

KeywordInhibition Of Ag3po4 Photocorrosion Ag3po4@mgfe2o4 Composites Rhb Degradation Visible Light-driven Possible Mechanism
Subject Area环境材料与生态化学
DOI10.1016/j.jallcom.2017.11.245
Funding Organizationthe National Natural Science Foundation of China (Grant No. 51768031) ; the key Research and Development Program in Gansu Province (Grant No. 17YF1NA056) ; the earmarked fund for Modern Agro-industry Technology Research System (Grant No. nycytx-15) ; Open Research Fund Program of Key Laboratory of Urban Stormwater System and Water Environment (Beijing University of Civil Engineering and Architecture), Ministry of Education (515205)
Indexed BySCI
If3.779
Language英语
Funding Project材料与农业工程组
compositor第二作者单位
Citation statistics
Cited Times:37[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.licp.cn/handle/362003/23800
Collection环境材料与生态化学研究发展中心
Corresponding AuthorZhang, Guozhen
Affiliation1.Lanzhou Jiaotong Univ, Sch Environm & Municipal Engn, Lanzhou 730070, Gansu, Peoples R China
2.Chinese Acad Sci, Lanzhou Inst Chem Phys, Res & Dev Ctr Ecomat & Ecochem, Lanzhou 730000, Gansu, Peoples R China
3.Beijing Univ Civil Engn & Architecture, Minist Educ, Key Lab Urban Stormwater Syst & Water Environm, Beijing, Peoples R China
Recommended Citation
GB/T 7714
Zhou TH,Zhang, Guozhen,Ma PJ,et al. Efficient degradation of rhodamine B with magnetically separable Ag3PO4@MgFe2O4 composites under visible irradiation[J]. Journal of Alloys and Compounds,2018,735(0):1277-1290.
APA Zhou TH.,Zhang, Guozhen.,Ma PJ.,Qiu XL.,Zhang, Hongwei.,...&Liu G.(2018).Efficient degradation of rhodamine B with magnetically separable Ag3PO4@MgFe2O4 composites under visible irradiation.Journal of Alloys and Compounds,735(0),1277-1290.
MLA Zhou TH,et al."Efficient degradation of rhodamine B with magnetically separable Ag3PO4@MgFe2O4 composites under visible irradiation".Journal of Alloys and Compounds 735.0(2018):1277-1290.
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