Peculiar synergetic effect of MoS2 quantum dots and graphene on Metal-Organic Frameworks for photocatalytic hydrogen evolution | |
Department | ERC国家工程研究中心 |
Hao, Xuqiang1,3; Jin ZL(靳治良)1; Yang, Hao1; Lu GX(吕功煊)2; Bi YP(毕迎普)2; Jin ZL(靳治良) | |
The second department | erc国家工程研究中心 |
2017 | |
Source Publication | Applied Catalysis B: Environmental |
ISSN | 0926-3373 |
Volume | 210Pages:45-56 |
Abstract | Special enhanced synergetic effect of MoS2 quantum dots (MoS2 QDs) and graphene on metal-organic frameworks for photocatalytic hydrogen evolution is obtained here. The photocatalytic activity of H2 evolution reach 186.37 mu mol over the EY-sensitized 5 rift% MoS2 QDs/UiO-66-NH2/G irradiated under visible light irradiation (λ ≥ 420nm) in the first 3 h, and the apparent quantum efficiency (AQE) is 40.5% at 430 nm. The synergistic effect between MoS2 QDs and graphene together with UiO-66-NH2 is corroborated by photo-luminescence spectra, electro-chemical and photo-electro-chemical experiments. It demonstrate that the charge separation and the electrons transfer are more efficient with the aid of the MoS2 QDs and graphene. MoS2 QDs might be a potential photocatalyst for design new type of catalysts in photocatalysis proton reduction. |
Keyword | Mos2 Qds Metal-organic Frameworks Graphene Photocatalytic Hydrogen Evolution |
Subject Area | 物理化学与绿色催化 |
DOI | 10.1016/j.apcatb.2017.03.057 |
Funding Organization | the Chinese National Natural Science Foundation (21603274;21263001;41663012;21433007) |
Indexed By | SCI |
If | 9.446 |
Language | 英语 |
Funding Project | 环境催化与氢能研究组;能源与环境纳米催化材料研究组 |
compositor | 第二作者单位 |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.licp.cn/handle/362003/22175 |
Collection | 羰基合成与选择氧化国家重点实验室(OSSO) 精细石油化工中间体国家工程研究中心(ERC) |
Corresponding Author | Jin ZL(靳治良) |
Affiliation | 1.Beifang Univ Nationalities, Sch Chem & Chem Engn, Yinchuan 750021, Peoples R China 2.Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Oxo Synth & Select Oxidat, Lanzhou 730000, Peoples R China 3.Nanjing Univ, Sch Chem & Chem Engn, Nanjing 210023, Jiangsu, Peoples R China |
Recommended Citation GB/T 7714 | Hao, Xuqiang,Jin ZL,Yang, Hao,et al. Peculiar synergetic effect of MoS2 quantum dots and graphene on Metal-Organic Frameworks for photocatalytic hydrogen evolution[J]. Applied Catalysis B: Environmental,2017,210:45-56. |
APA | Hao, Xuqiang,Jin ZL,Yang, Hao,Lu GX,Bi YP,&靳治良.(2017).Peculiar synergetic effect of MoS2 quantum dots and graphene on Metal-Organic Frameworks for photocatalytic hydrogen evolution.Applied Catalysis B: Environmental,210,45-56. |
MLA | Hao, Xuqiang,et al."Peculiar synergetic effect of MoS2 quantum dots and graphene on Metal-Organic Frameworks for photocatalytic hydrogen evolution".Applied Catalysis B: Environmental 210(2017):45-56. |
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