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3D hierarchical WO3 grown on TiO2 nanotube arrays and their photoelectrochemical performance for water splitting
Department固体润滑国家重点实验室
Sun WX(孙炜翔)1,2; Wang DA(王道爱)2; Zia Ur Rahman2; Wei N(卫宁)1,2; Chen,Shougang1; Wang DA(王道爱)
2016
Source PublicationJournal of Alloys and Compounds
ISSN0925-8388
Volume695Pages:2154-2159
Abstract

WO3 with 3D hierarchical structure was successfully grown into the TiO2 nanotube arrays (TiO2 NTs) on Ti substrate by two-steps procedure. First, TiO2 NTs were fabricated through anodization of titanium, and then WO3 nanoparticles were deposited into the TiO2 NTs and the WO3 with 3D hierarchical structures were deposited on the top surface of TiO2 NTs through hydrothermal method. The WO3/TiO2 composite photoelectrode showed better photoelectric response in visible light compared with the pristine TiO2 and WO3 electrodes. A higher photocurrent density was achieved by optimizing the experimental conditions including solution concentration, hydrothermal time and reaction temperature in details. The improvement of photoelectrochemical (PEC) response for WO3/TiO2 composite photoelectrode also indicated an important synergy between visible light absorption and 3D hierarchical structure inherent to WO3 and the new formed semiconductor composite structures fabricated by hydrothermal treatment, which offers a significant improvement in the separation and transmission of photo generated electrons.

KeywordTungsten Oxide Titania Nanotube Hydrothermal Photoelectrochemical Performance
Subject Area材料科学与物理化学
DOI10.1016/j.jallcom.2016.11.061
Funding Organizationthe NSFC (21303227;21573259);Qingdao science and technology plan application foundation research project (14-2-4-60-JCH);the “Hundred Talents Program” of Chinese Academy of Sciences (D. Wang)
Indexed BySCI
If3.133
Language英语
Funding Project材料表面与界面行为研究组
compositor第二作者单位
Citation statistics
Cited Times:22[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.licp.cn/handle/362003/20602
Collection固体润滑国家重点实验室(LSL)
Corresponding AuthorChen,Shougang; Wang DA(王道爱)
Affiliation1.Institute of Material Science and Engineering, Ocean University of China, Qingdao 266100, China
2.Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China
Recommended Citation
GB/T 7714
Sun WX,Wang DA,Zia Ur Rahman,et al. 3D hierarchical WO3 grown on TiO2 nanotube arrays and their photoelectrochemical performance for water splitting[J]. Journal of Alloys and Compounds,2016,695:2154-2159.
APA Sun WX,Wang DA,Zia Ur Rahman,Wei N,Chen,Shougang,&王道爱.(2016).3D hierarchical WO3 grown on TiO2 nanotube arrays and their photoelectrochemical performance for water splitting.Journal of Alloys and Compounds,695,2154-2159.
MLA Sun WX,et al."3D hierarchical WO3 grown on TiO2 nanotube arrays and their photoelectrochemical performance for water splitting".Journal of Alloys and Compounds 695(2016):2154-2159.
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