Pulsed laser deposition of CuInS2 quantum dots on one-dimensional TiO2 nanorod arrays and their photoelectrochemical characteristics | |
Department | 固体润滑国家重点实验室 |
Han MM(韩敏敏)1,2; Chen WY(陈文元)1,2; Guo HJ(国洪建)1,2; Yu LM(于丽敏)1,2; Li B(李波)1; Jia JH(贾均红)1; Jia JH(贾均红) | |
2016 | |
Source Publication | Journal of Power Sources |
ISSN | 0378-7753 |
Volume | 318Pages:121-127 |
Abstract | In the typical solution-based synthesis of colloidal quantum dots (QDs), it always resorts to some surface treatment, ligand exchange processing or post-synthesis processing, which might involve some toxic chemical regents injurious to the performance of QD sensitized solar cells. In this work, the CuInS2 QDs are deposited on the surface of one-dimensional TiO2 nanorod arrays by the pulsed laser deposition (PLD) technique. The CuInS2 QDs are coated on TiO2 nanorods without any ligand engineering, and the performance of the obtained CuInS2 QD sensitized solar cells is optimized by adjusting the laser energy. An energy conversion efficiency of 3.95% is achieved under one sun illumination (AM 1.5, 100 mW cm−2). The improved performance is attributed to enhanced absorption in the longer wavelength region, quick interfacial charge transfer and few chance of carrier recombination with holes for CuInS2 QD-sensitized solar cells. Moreover, the photovoltaic device exhibits high stability in air without any specific encapsulation. Thus, the PLD technique could be further applied for the fabrication of QDs or other absorption materials. |
Keyword | Cuins2 Quantum Dots Sensitized Solar Cells Pulsed Laser Deposition Technique Interfacial Charge Transfer Carrier Recombination |
Subject Area | 材料科学与物理化学 |
DOI | 10.1016/j.jpowsour.2016.04.011 |
Funding Organization | the National Natural Science Foundation of China (Grant No. 51471181;51175490) |
Indexed By | SCI |
If | 6.395 |
Language | 英语 |
Funding Project | 高温抗磨材料组 |
compositor | 第一作者单位 |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.licp.cn/handle/362003/20102 |
Collection | 固体润滑国家重点实验室(LSL) |
Corresponding Author | Jia JH(贾均红) |
Affiliation | 1.Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100080, Peoples R China |
Recommended Citation GB/T 7714 | Han MM,Chen WY,Guo HJ,et al. Pulsed laser deposition of CuInS2 quantum dots on one-dimensional TiO2 nanorod arrays and their photoelectrochemical characteristics[J]. Journal of Power Sources,2016,318:121-127. |
APA | Han MM.,Chen WY.,Guo HJ.,Yu LM.,Li B.,...&贾均红.(2016).Pulsed laser deposition of CuInS2 quantum dots on one-dimensional TiO2 nanorod arrays and their photoelectrochemical characteristics.Journal of Power Sources,318,121-127. |
MLA | Han MM,et al."Pulsed laser deposition of CuInS2 quantum dots on one-dimensional TiO2 nanorod arrays and their photoelectrochemical characteristics".Journal of Power Sources 318(2016):121-127. |
Files in This Item: | ||||||
File Name/Size | DocType | Version | Access | License | ||
1-s2.0-S037877531630(2008KB) | 期刊论文 | 作者接受稿 | 开放获取 | CC BY-NC-SA | View Application Full Text |
Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.
Edit Comment